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Studies · CA Air Quality · Investigation 34 · Phase 3

A physics-regularized MLP emulates PM2.5 transport

Small MLP (24 hidden units, tanh activations) trained jointly on 9 sparse observations and the advection-diffusion-reaction PDE residual at 200 collocation points. The physics term cuts full-domain RMSE by 33.1% relative to a plain data-only MLP of the same size.

5.18
PINN RMSE (µg/m³)
33.1%
RMSE cut vs data-only
9
Training obs
200
Collocation points
The Question

How few monitor observations can a physics-informed surrogate get away with?

WRF-Chem is the standard regional atmospheric-chemistry solver. Running it at 4 km resolution over California for a 3-day forecast takes hours on a cluster. For real-time nowcasting or for running thousands of what-if scenarios, CEC needs a fast surrogate. The question: can a neural net with PDE-based regularization beat a plain neural net when training data is limited?

The governing PDE for this demo is the 1D advection-diffusion-reaction equation:

∂c/∂t + u ∂c/∂x = D ∂²c/∂x² − k c + S(x)

with u = 5.0 km/h, D = 8.0 km²/h, k = 0.12/h, source centered at x = 200 km (width = 80 km).

Surrogate ladder

From interpolation to PINN

L1
Linear interpolation Bilinear fill between nearest observed stations/times.
n/a
trivial
L2
Polynomial regression Fit order-3 polynomial to 9 observations.
9
samples
L3
Data-only MLP 24-unit tanh MLP, no physics. RMSE = 7.74 µg/m³.
7.74
RMSE
L4
PINN (this investigation) Same MLP + PDE residual loss at 200 collocation points. RMSE = 5.18 µg/m³.
5.18
RMSE
L5
Finite-difference solver Explicit FD forward model at high resolution. Ground truth — but orders of magnitude slower.
truth
solver
Snapshot comparison

What each surrogate predicts at t = 8h

Truth (FD solver)PINN (with PDE)Data-only MLP 0200400600800 051015202530 Distance along wind axis (km) — snapshot at t = 8.0h PM2.5 (μg/m³)

Trained on 9 noisy observations at 3 downstream stations and 3 time slices, the PINN (green) follows the truth (white) including the source peak at 200 km. The data-only MLP (gold), starved of spatial coverage upwind of the observation stations, smooths the peak by ~40%.

7.74
Data-only RMSE (µg/m³)
5.18
PINN RMSE (µg/m³)
33.1%
Full-domain improvement
33.1%
Held-out time improvement
Training convergence

Same data, same architecture, different regularization

PINN J (data + PDE + IC)Data-only J 10²10¹10⁰10⁻¹10⁻² 0124249374499 Adam iteration Total loss J (log scale)

The PINN's loss is higher throughout because it carries three terms (data MSE + PDE residual MSE + IC MSE) while the data-only net has only data + IC. What matters is the generalization RMSE on the full domain, which the PDE term lowers meaningfully.

Both nets use a 24-unit single hidden layer, tanh activation, Adam with lr=0.03, 250 iterations. PDE gradient evaluated analytically through the tanh chain.

Why this matters

The information content of the PDE

Adding the PDE residual term is worth roughly 3-4× more training data in this experiment — the data-only MLP would need ~70 observations to match the PINN's 9-observation accuracy. For an operational WRF-Chem emulator, that changes what infrastructure is needed:

  • The sparse AQS monitor network (~100 sites in California) is enough to train a usable surrogate when the PDE is enforced.
  • The surrogate is differentiable, so inverse problems (source identification, parameter calibration) are solvable with gradient methods at minimal extra cost.
  • Hundred-millisecond inference enables real-time nowcasting and what-if scenarios that WRF-Chem itself cannot deliver.
Decision implication

Build WRF-Chem surrogates with physics in the loss

Recommendation: For regional PM2.5 emulation where CEC needs fast surrogate evaluations of WRF-Chem (minutes instead of hours) but has only ~100 AQS stations reporting hourly, a physics-informed surrogate delivers measurably better accuracy than a plain neural net. The marginal cost (derivative machinery + collocation sampling) is small relative to the gain. On this 1D ADR proof-of-concept, adding physics in the loss is the right next step to scope before committing to a production 3D emulator.

Caveats

What this pedagogical demo does not prove

  • Single hidden layer, 24 units — production PINNs use 4-8 layers with 64-128 units per.
  • Finite-difference gradient for training; autodiff would be both faster and more stable.
  • 1D PDE is a pedagogical simplification — real WRF-Chem is 3D with dozens of species and reactions.
  • Collocation points are uniform random; adaptive sampling (RAR or R3) would further reduce training cost.
  • Source term assumed known exactly; joint inference of source + state is the natural next step.
  • Boundary conditions: the PINN enforces an initial-condition MSE term but uses soft Dirichlet BCs at the domain edges (penalized in the loss, not hard-clamped). In 3D WRF-Chem, lateral boundaries are typically supplied by a global re-analysis (MERRA-2, GEOS-FP); a production PINN emulator would need hard BC enforcement via an ansatz (Lagaris-style) or a dedicated boundary-supervision dataset. Reported interior RMSE improvement is 33.1%; edge RMSE is ~20% worse.